Ryder, C. L., Highwood, E. J., Rosenberg, P. D., Trembath, J., Brooke, J. K., Bart, M., Dean, A., Crosier, J., Dorsey, J., Brindley, H., Banks, J., Marsham, J. H., McQuaid, J. B., Sodemann, H. and Washington, R.
Optical properties of Saharan dust aerosol and contribution from the coarse mode as measured during the Fennec 2011 aircraft campaign.
Atmospheric Chemistry and Physics, 13 (1).
To link to this item DOI: 10.5194/acp-13-303-2013
New in-situ aircraft measurements of Saharan dust
originating from Mali, Mauritania and Algeria taken during
the Fennec 2011 aircraft campaign over a remote part of
the Sahara Desert are presented. Size distributions extending to 300 μm are shown, representing measurements extending further into the coarse mode than previously published for airborne Saharan dust. A significant coarse mode was present in the size distribution measurements with effective diameter (deff) from 2.3 to 19.4 μm and coarse mode volume median diameter (dvc) from 5.8 to 45.3 μm. The mean size distribution had a larger relative proportion of coarse mode particles than previous aircraft measurements. The largest particles (with deff >12 μm, or dvc >25 μm) were only encountered within 1 km of the ground. Number concentration, mass loading and extinction coefficient showed inverse relationships to dust age since uplift. Dust particle size showed a weak exponential relationship to dust age. Two cases of freshly uplifted dust showed quite different characteristics of size distribution and number concentration.
Single Scattering Albed (SSA) values at 550 nm calculated
from the measured size distributions revealed high absorption ranging from 0.70 to 0.97 depending on the refractive index. SSA was found to be strongly related to deff. New instrumentation revealed that direct measurements, behind Rosemount inlets, overestimate SSA by up to 0.11 when
deff is greater than 2 μm. This is caused by aircraft inlet inefficiencies and sampling losses. Previous measurements of
SSA from aircraft measurements may also have been overestimates for this reason. Radiative transfer calculations indicate that the range of SSAs during Fennec 2011 can lead to underestimates in shortwave atmospheric heating rates by 2.0 to 3.0 times if the coarse mode is neglected. This will have an impact on Saharan atmospheric dynamics and circulation,which should be taken into account by numerical weather prediction and climate models.
|Date Deposited:||20 Nov 2014 09:56|
|Last Modified:||19 Feb 2017 08:56|
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